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Activity Ordering

Alternatively, we may order the orbitals according to their ``activity'' (i.e. frozen, occupied, unoccupied, etc). The Quantum Trio standard order calls for all frozen core orbitals to come first, then all doubly-occupied orbitals, then all singly-occupied orbitals, then unoccupied active orbitals, and finally all frozen virtual orbitals. Within each major section, orbitals are numbered according to irreducible representation. Within each irrep, orbitals are numbered according to energy (if they are molecular orbitals).gif This is particularly useful in, for instance, a CI calculation. Since all frozen core orbitals have consecutive indices, removing the core orbitals from explicit consideration in the correlated wavefunction simply means starting the loops over orbitals with the first active orbital. Likewise, removing the frozen virtual orbitals means tossing out all orbitals with an index greater than that of the last active orbital. Loops over occupied and virtual orbitals are also easier to deal with since the orbitals in each of these groups are numbered consecutively.



© 1996 by C. David Sherrill  / sherrill@bastille.cchem.berkeley.edu
Last modified: Tue Sep 17 22:13:09 EDT 1996